1. Disturbed, upset.
    I was unsettled by the sudden outburst, and since I didn't know what to do I just stood there, confused.
  2. Not in a steady condition, uncertain, subject to change.
  3. Not populated, having no settlers or other inhabitants.
  4. Unpaid.
    We need to settle this bill; even if you think the charge is too high we can't just leave it unsettled.
  1. Simple past tense and past participle of unsettle

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